Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition
It is well established that the performance of LED and laser devices can be enhanced by optimizing the heat sink. Aluminum oxide (Al2O3) is one of the most effective materials for use as a heat sink. In this study, YAG: Ce3+ thin films were deposited onto sapphire substrates with a (0001) orientatio...
Сохранить в:
| Главные авторы: | , , , |
|---|---|
| Формат: | Статья |
| Язык: | English |
| Опубликовано: |
Elsevier Ltd
2025
|
| Темы: | |
| Online-ссылка: | https://dspace.ncfu.ru/handle/123456789/29814 |
| Метки: |
Добавить метку
Нет меток, Требуется 1-ая метка записи!
|
| id |
ir-123456789-29814 |
|---|---|
| record_format |
dspace |
| spelling |
ir-123456789-298142025-02-20T13:34:58Z Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition Devitsky, O. V. Девицкий, О. В. Kravtsov, A. A. Кравцов, А. А. Annealing Thin films Photoluminescence Ce Pulsed laser deposition YAG X-ray diffraction It is well established that the performance of LED and laser devices can be enhanced by optimizing the heat sink. Aluminum oxide (Al2O3) is one of the most effective materials for use as a heat sink. In this study, YAG: Ce3+ thin films were deposited onto sapphire substrates with a (0001) orientation using pulsed laser deposition method. It was observed that the annealing temperature did not significantly affect the thickness of the films, but it did influence their uniformity and structure. As the annealing temperature of the YAG: Ce films increased, crystallite growth was noted. The polydispersity of the grains also increased with higher annealing temperatures, indicating competitive growth phenomena. Raising the annealing temperature to 1400 °C led to the formation of gaps in the film structure due to recrystallization processes. Luminescence measurements revealed that, despite the structural differences among films annealed at various temperatures, their emission spectra remained consistent with the target. This suggests the stability of the energy structure of YAG: Ce and the successful transfer of YAG stoichiometry during the pulsed laser deposition process. As a result, optimal conditions for the thermal annealing of YAG: Ce thin films were identified, leading to high crystalline perfection and the formation of a heteroepitaxial interface with the Al2O3 (0001) substrate. This finding is potentially significant for enhancing the thermal characteristics of composite structures. 2025-02-20T13:34:09Z 2025-02-20T13:34:09Z 2025 Статья Devitsky O.V., Kravtsov A.A. Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition // Ceramics International. - 2025. - 51 (5). - pp. 6011 - 6022. - DOI: 10.1016/j.ceramint.2024.12.047 https://dspace.ncfu.ru/handle/123456789/29814 en Ceramics International application/pdf application/pdf Elsevier Ltd |
| institution |
СКФУ |
| collection |
Репозиторий |
| language |
English |
| topic |
Annealing Thin films Photoluminescence Ce Pulsed laser deposition YAG X-ray diffraction |
| spellingShingle |
Annealing Thin films Photoluminescence Ce Pulsed laser deposition YAG X-ray diffraction Devitsky, O. V. Девицкий, О. В. Kravtsov, A. A. Кравцов, А. А. Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| description |
It is well established that the performance of LED and laser devices can be enhanced by optimizing the heat sink. Aluminum oxide (Al2O3) is one of the most effective materials for use as a heat sink. In this study, YAG: Ce3+ thin films were deposited onto sapphire substrates with a (0001) orientation using pulsed laser deposition method. It was observed that the annealing temperature did not significantly affect the thickness of the films, but it did influence their uniformity and structure. As the annealing temperature of the YAG: Ce films increased, crystallite growth was noted. The polydispersity of the grains also increased with higher annealing temperatures, indicating competitive growth phenomena. Raising the annealing temperature to 1400 °C led to the formation of gaps in the film structure due to recrystallization processes. Luminescence measurements revealed that, despite the structural differences among films annealed at various temperatures, their emission spectra remained consistent with the target. This suggests the stability of the energy structure of YAG: Ce and the successful transfer of YAG stoichiometry during the pulsed laser deposition process. As a result, optimal conditions for the thermal annealing of YAG: Ce thin films were identified, leading to high crystalline perfection and the formation of a heteroepitaxial interface with the Al2O3 (0001) substrate. This finding is potentially significant for enhancing the thermal characteristics of composite structures. |
| format |
Статья |
| author |
Devitsky, O. V. Девицкий, О. В. Kravtsov, A. A. Кравцов, А. А. |
| author_facet |
Devitsky, O. V. Девицкий, О. В. Kravtsov, A. A. Кравцов, А. А. |
| author_sort |
Devitsky, O. V. |
| title |
Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| title_short |
Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| title_full |
Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| title_fullStr |
Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| title_full_unstemmed |
Effect of thermal annealing on the structural evolution of thin ceramic YAG: Ce films grown by pulsed laser deposition |
| title_sort |
effect of thermal annealing on the structural evolution of thin ceramic yag: ce films grown by pulsed laser deposition |
| publisher |
Elsevier Ltd |
| publishDate |
2025 |
| url |
https://dspace.ncfu.ru/handle/123456789/29814 |
| work_keys_str_mv |
AT devitskyov effectofthermalannealingonthestructuralevolutionofthinceramicyagcefilmsgrownbypulsedlaserdeposition AT devickijov effectofthermalannealingonthestructuralevolutionofthinceramicyagcefilmsgrownbypulsedlaserdeposition AT kravtsovaa effectofthermalannealingonthestructuralevolutionofthinceramicyagcefilmsgrownbypulsedlaserdeposition AT kravcovaa effectofthermalannealingonthestructuralevolutionofthinceramicyagcefilmsgrownbypulsedlaserdeposition |
| _version_ |
1842245721443532800 |